Raids in 28 locations in the southern cities of Granada, Málaga and Seville earlier this month netted caches of money and weapons, as well as 10 luxury vehicles and over two tonnes of marijuana, Spain's Guardia Civil police force said.
Officers arrested 36 suspects from 10 nations as part of the operation, including the suspected leader of the network, a man of Turkish origin who lived in Spain and was the target of an international arrest warrant issued by Turkey, they added.
The group "was focused on exporting large amounts of marijuana and heroin from our country to Germany and other nations in Eastern Europe", police said.
The arrested suspects also included nationals from Argentina, Austria, Germany, Montenegro, Romania, Spain, Syria, Ukraine and Venezuela.
European Union police force Europol, which coordinated the investigation, said over 400 officers from French, Spanish and Turkish law enforcement agencies took part in the operation.
Spain is one of the main entry points for drugs into Europe given its close ties with Latin America and its proximity to Morocco.
Latin America is the main source of cocaine and Morocco is a key source of hashish, a sticky brown substance made from the resin of the cannabis plant.
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